In the synthesized form, the crystalline material has acomposition, in terms of moles of anhydrous oxides per 100 moles of tetravalent element oxide as follows:wherein X and Y are as defined above, M is an alkali or alkaline earth metal, n is the valence of M, and R' and R are the directing agents tetramethyl ammonium hydroxide (TMAOH) and quinuclidine, respectively.The original alkali or alkalin